Classic resource recommenders like Collaborative Filtering treat users as just another entity, thereby neglecting non-linear user-resource dynamics that shape attention and interpretation. SUSTAIN, as an unsupervised hu- man category learning model, captures these dynamics. It aims to mimic a learner's categorization behavior. In this paper, we use three social bookmarking datasets gathered from BibSonomy, CiteULike and Delicious to investigate SUSTAIN as a user modeling approach to re-rank and enrich Collaborative Filtering following a hybrid recommender strategy. Evaluations against baseline algorithms in terms of recommender accuracy and computational complexity reveal encouraging results. Our approach substantially improves Collaborative Filter- ing and, depending on the dataset, successfully competes with a computationally much more expensive Matrix Factorization variant. In a further step, we explore SUSTAIN's dynamics in our specific learning task and show that both memorization of a user's history and clustering, contribute to the algorithm's performance. Finally, we observe that the users' attentional foci determined by SUSTAIN correlate with the users' level of curiosity, identified by the SPEAR algorithm. Overall, the results of our study show that SUSTAIN can be used to efficiently model attention-interpretation dynamics of users and can help improve Collaborative Filtering for resource recommendations.